Search results for "Non polar"
showing 7 items of 7 documents
Gas—liquid chromatographic analyses
1984
Abstract The gas chromatography (GC) of n -alkyl acetates (CH 3 COOR), chloroacetates (CH 2 ClCOOR), dichloroacetates (CHCl 2 COOR) and trichloroacetates (CCl 3 COOR), where the alcohol chain length (R) varied between 1 and 8, and certain of their monochlorinated derivatives, 176 compounds altogether, has been studied on SE-30 and OV-351 glass capillary columns under the same operating conditions. The isomeric monochlorinated esters are eluted in direct order from the 1- chloro to the ω-chloro isomer, the separation of the isomers being complete on OV- 351. On SE-30, however, the peaks of the 6- and 7-chlorooctyl esters are partly overlapped. The separation of the mixtures of odd- and e…
Gas-liquid chromatographic analyses
1984
A mixture of all nine chlorinated 4-hydroxybenzaldehydes and the parent homologue was separated on a non-polar SE-30 capillary column using various isothermal and temperature-programmed operating conditions. The relative retention data for the compounds are given and the retention indices together with the retention index increments for each position of chlorine substitution are examined. The retention order 3-Cl<parent<2,5-di-Cl<2,3-di-Cl<3,5-di-Cl<2-Cl<2,3,5-tri-Cl<2,3,6-tri-Cl<2,6-di-Cl<tetra-Cl isomer obtained indicates that the effect of the position of substitution on the retention behaviour is greater than that of the number of chlorine atoms. The retention is maximal with 2-Cl and 2…
Understanding the Origin of the Regioselectivity in Non-polar [3+2] Cycloaddition Reactions through the Molecular Electron Density Theory
2020
The regioselectivity in non-polar [3+2] cycloaddition (32CA) reactions has been studied within the Molecular Electron Density Theory (MEDT) at the B3LYP/6-311G(d,p) level. To this end, the 32CA reactions of nine simplest three-atom-components (TACs) with 2-methylpropene were selected. The electronic structure of the reagents has been characterized through the Electron Localisation Function (ELF) and the Conceptual DFT. The energy profiles of the two regioisomeric reaction paths and ELF topology of the transition state structures are studied to understand the origin of the regioselectivity in these 32CA reactions. This MEDT study permits to conclude that the least electronegative X1 end atom…
Collapsibility of metastable sand by non-conventional oedometer tests
2018
The stability of foundations soils could represent a clear and present threat for the conservation of even well preserved buildings, particularly for Architectural heritage conservation and land art heritage. A dramatic case is the presence of collapsible metastable sands as foundation soils, as it occurs in the sacral complex Valle dei Templi in Agrigento. This site listed by UNESCO, stands on a crest of a calcarenite cuesta, overlaying a layer of these sands. When the collapsible sand is dry, the structure is strong enough to bond the sand particles together. When the sand becomes wet, a de-structuration mechanism occurs and the soil’s strength is compromised. This paper has a twofold aim…
endo-Functionalized molecular tubes : selective encapsulation of neutral molecules in non-polar media
2016
Four endo-functionalized molecular tubes with urea/thiourea groups in the deep cavities have been synthesized, and their binding ability to neutral molecules studied. Very high binding affinity and selectivity have been achieved, which are rationalized by invoking the shape and electrostatic complementarity and dipole alignment.
Gas chromatography of homologous esters
1984
Abstract The gas chromatographic retention behaviour of the propanoyl and monochloropropanoyl esters of saturated C3C5 branched-chain and unsaturated C3C6 alcohols on SE-30 and OV-351 capillary columns at several temperatures is reported. Retention index increments at 80 and 120°C show the effect of branching in the alkyl chain and also the effect of unsaturation and of its position in the chain with chlorination at the two possible positions in the acyl chain. The various incremental effects are discussed and compared with the behaviour of the corresponding n-alkyl esters.
Time-dependent monomerization of gramicidin A, enhanced by phosphatidylcholine in non-polar solvents
1986
Abstract The usefulness of size-exclusion high-performance liquid chromatography for the study of gramicidin A dimer—monomer conformational equilibrium in non